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Yes

Fred Armisen as Brainy Smurf (voice)
Evan Sabara as Robin / Dick Grayson
Bridget Everett as Elena
Sean Giambrone as Travis (voice)
Antony Del Rio as Kyle
Saori Onishi as Yuki Sumi
Debi Derryberry as Additional Dialogue Replacement (voice)
Ryota Takeuchi as Tachibana Aoi
Adam Wylie as Panicky Smurf (voice)
Jun Fukushima as Tsav
Shin'ichirou Miki as Sig
Jun Fukushima as Chikara Ōta
Walter Jones as Additional Voices (voice)
Christina Ricci as Vexy (voice)
Matthew Wood as Additional Voices (voice)
Dave B. Mitchell as 1st Commercial Guy (voice)
Shun Horie as Albert
Andy Samberg as Baby Brent (voice)
Elizabeth Daily as Additional Voices (voice)
Jean Gilpin as ADR Group (voice)
Ian McShane as Agent D (voice)
ND Stevenson as Spinarella
Grace Helbig as Sugar Cookieloaf (voice)
B.J. Novak as Baker Smurf (voice)

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